The answer is quite simple, no you are not allowed to remove the clamps. A rafter roof is a system with foot points with horizontal and vertical supports with a ridge point as a hinge, e.g. as a lap joint or as in your case with a floating ridge purlin and the double clamps. Can you change it, yes, if you convert your rafter roof into a load-bearing purlin roof, which means purlins with supports arranged underneath. More or less sensible, as the purlins in terms of cross-sections will not be sufficient for the existing support spans, and you additionally need supports especially under the ridge purlin, which often get in the way and cause disturbance. Everything is possible but also very costly. But without an appropriate structural engineer, you won’t get by in this case.